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Title:Anharmonic quantum effects of implanted muons : route to probing nuclear quantum behavior in solids
Authors:ID Hotz, Fabian (Author)
ID Gomilšek, Matjaž, Institut "Jožef Stefan" (Author)
ID Arh, Tina (Author)
ID Hicken, Thomas (Author)
ID Umek, Polona, Institut "Jožef Stefan" (Author)
ID Zorko, Andrej, Institut "Jožef Stefan" (Author)
ID Luetkens, Hubertus (Author)
Files:URL URL - Source URL, visit https://journals.aps.org/prb/pdf/10.1103/x1y3-9chs
 
.pdf PDF - Presentation file, download (2,23 MB)
MD5: 5C1180907A5DB3801D9FD800BFD3410E
 
Language:English
Typology:1.01 - Original Scientific Article
Organization:Logo IJS - Jožef Stefan Institute
Abstract:The quantum behavior of light particles in solids gives rise to phenomena that cannot be captured by a classical description. We show that muon spin spectroscopy (μSR), when paired with a quantum-mechanical treatment of the implanted muon, becomes a sensitive and direct probe of nuclear quantum effects. By modeling the muon as a spatially extended quantum particle, our approach captures strong anharmonic behavior. We demonstrate this in Zn-barlowite, which serves as a nontrivial test case due to its structurally complex lattice and the presence of both fluorine and hydroxyl groups. Our results establish a route for extracting nuclear quantum signatures from μSR data and open different opportunities for studying light nuclei such as hydrogen and lithium in systems where quantum fluctuations shape structure and function.
Keywords:defects, magnetic interactions, magnetization dynamics, spin dynamics, density functional theory, muon spin resonance
Publication status:Published
Publication version:Version of Record
Submitted for review:17.07.2025
Article acceptance date:07.04.2026
Publication date:08.06.2026
Publisher:American Physical Society
Year of publishing:2026
Number of pages:str. 224420-1-224420-8
Numbering:Vol. 113, [article no.] 224420
Source:ZDA
PID:20.500.12556/DiRROS-30306 New window
UDC:539.1
ISSN on article:2469-9969
DOI:10.1103/x1y3-9chs New window
COBISS.SI-ID:281774083 New window
Note:Nasl. z nasl. zaslona; Soavtorji iz Slovenije: M. Gomilšek, P. Umek, A. Zorko; Opis vira z dne 16. 6. 2026;
Publication date in DiRROS:19.06.2026
Views:42
Downloads:34
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Record is a part of a journal

Title:Physical review
Shortened title:Phys. rev. B.
Publisher:American Physical Society
ISSN:2469-9969
COBISS.SI-ID:3042148 New window

Document is financed by a project

Funder:SNSF - Swiss National Science Foundation
Project number:192109
Name:Stabilization and destabilization of spin liquids by perturbations

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:P1-0125-2022
Name:Fizika kvantnih in funkcionalnih materialov

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:Z1-1852-2019
Name:Raziskave frustriranih skirmionov z jedrsko magnetno resonanco

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:N1-0148-2020
Name:Stabilizacija in destabilizacija spinskih tekočin zaradi perturbacij

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:J1-2461-2020
Name:Nova eksperimentalna metoda določitve kvantnih spinskih tekočin

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:J1-50008-2023
Name:Anizotropen kvantni magnetizem novih materialov z redkimi zemljami

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:J1-50012-2023
Name:Prepletena in delokalizirana staja mionov in jeder

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:N1-0356-2024
Name:Kvantni pojavi lahkih delcev v snovi

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:N1-0345-2024
Name:Razvoj kompleksnim magnetnih in polarnih redov iz enostavnih 2D podstruktur v plastovitih hidridnih organo-anorganskih halogenometalatih

Funder:ARIS - Slovenian Research and Innovation Agency
Project number:J2-60034-2025
Name:Praktična kvantna prednost računanja z rezervoarji na NISQ napravah

Licences

License:CC BY 4.0, Creative Commons Attribution 4.0 International
Link:http://creativecommons.org/licenses/by/4.0/
Description:This is the standard Creative Commons license that gives others maximum freedom to do what they want with the work as long as they credit the author.
Licensing start date:08.06.2026
Applies to:VoR

Secondary language

Language:Slovenian
Keywords:defekti, magnetne interakcije, dinamika magnetizacije, spinova dinamika, teorija gostotnega funkcionala, mionska spinovna resonanca


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